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Article: Control of electron localization in molecular dissociation

TitleControl of electron localization in molecular dissociation
Authors
Kling, M. F.Siedschlag, ChVerhoef, A. J.Khan, J. I.Schultze, M.Uphues, ThNi, Y.Uiberacker, M.Drescher, M.Krausz, F.Vrakking, M. J.J.
Issue Date2006
Citation
Science, 2006, v. 312, n. 5771, p. 246-248 How to Cite?
DOI: http://dx.doi.org/10.1126/science.1126259
AbstractWe demonstrated how the subcycle evolution of the electric field of light can be used to control the motion of bound electrons. Results are presented for the dissociative ionization of deuterium molecules (D2 → D + + D), where asymmetric ejection of the ionic fragment reveals that light-driven intramolecular electronic motion before dissociation localizes the electron on one of the two D+ ions in a controlled way. The results extend subfemtosecond electron control to molecules and provide evidence of its usefulness in controlling reaction dynamics.
Persistent Identifierhttp://hdl.handle.net/10722/364417
ISSN
0036-8075
2023 Impact Factor: 44.7
2023 SCImago Journal Rankings: 11.902

 

DC FieldValueLanguage
dc.contributor.authorKling, M. F.-
dc.contributor.authorSiedschlag, Ch-
dc.contributor.authorVerhoef, A. J.-
dc.contributor.authorKhan, J. I.-
dc.contributor.authorSchultze, M.-
dc.contributor.authorUphues, Th-
dc.contributor.authorNi, Y.-
dc.contributor.authorUiberacker, M.-
dc.contributor.authorDrescher, M.-
dc.contributor.authorKrausz, F.-
dc.contributor.authorVrakking, M. J.J.-
dc.date.accessioned2025-10-30T08:33:36Z-
dc.date.available2025-10-30T08:33:36Z-
dc.date.issued2006-
dc.identifier.citationScience, 2006, v. 312, n. 5771, p. 246-248-
dc.identifier.issn0036-8075-
dc.identifier.urihttp://hdl.handle.net/10722/364417-
dc.description.abstractWe demonstrated how the subcycle evolution of the electric field of light can be used to control the motion of bound electrons. Results are presented for the dissociative ionization of deuterium molecules (D<inf>2</inf> → D <sup>+</sup> + D), where asymmetric ejection of the ionic fragment reveals that light-driven intramolecular electronic motion before dissociation localizes the electron on one of the two D<sup>+</sup> ions in a controlled way. The results extend subfemtosecond electron control to molecules and provide evidence of its usefulness in controlling reaction dynamics.-
dc.languageeng-
dc.relation.ispartofScience-
dc.titleControl of electron localization in molecular dissociation-
dc.typeArticle-
dc.description.naturelink_to_subscribed_fulltext-
dc.identifier.doi10.1126/science.1126259-
dc.identifier.scopuseid_2-s2.0-33645834950-
dc.identifier.volume312-
dc.identifier.issue5771-
dc.identifier.spage246-
dc.identifier.epage248-
dc.identifier.eissn1095-9203-

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