Spatial-and-local-aware deep learning approach for Ground-Level NO2 estimation in England with multisource data from satellite-based observations and chemical transport models

Abstract

<p>High-resolution near-surface NO2 data are crucial for monitoring air pollution dynamics. Satellite-based machine learning models are commonly used to estimate NO2 concentrations, but tailoring advanced deep learning techniques to specific environmental problems remains challenging. This study applies a two-stage deep learning approach to estimate ground-level NO2 concentrations in England at a 1 km spatial resolution from 2019 to 2021. Initially, we imputed the TROPOMI NO2 column density to a continuous 1 km resolution. We then developed an efficient spatial-and-local-aware deep learning network (SLNet) for NO2 mapping by integrating the imputed TROPOMI NO2 data with multi-source information from meteorology, chemical transport model (CTM) simulations, and other auxiliary predictors. To address the translation invariance of convolutional neural networks (CNNs), we combined a local channel to identify spatial heterogeneity in the model. Our imputed TROPOMI NO2 surfaces, which initially covered only 34.12 % of valid data, achieved full coverage with reliability and continuity at 1 km spatial resolution. Cross-validation confirmed that the SLNet model outperformed other state-of-the-art methods in estimating ground-level NO2. The prediction model achieved R² values of 0.914, 0.919, and 0.887 for 2019, 2020, and 2021, respectively, and performed well in urban regions. Additionally, the Shapley Additive Explanations (SHAP) method revealed that features such as satellite and CTM NO2, precipitation, green space, and road density significantly contributed to estimations through both spatial and local channels. The mapping results closely aligned with ground-level observations and accurately captured spatial variations. This study advances NO2 concentration estimation by applying adaptable deep learning techniques and enhances the understanding of air pollution dynamics.</p>