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Article: In-situ synthesis of heterojunction TiO2/MnO2 nanostructure with excellent performance in vacuum ultraviolet photocatalytic oxidation of toluene

TitleIn-situ synthesis of heterojunction TiO2/MnO2 nanostructure with excellent performance in vacuum ultraviolet photocatalytic oxidation of toluene
Authors
KeywordsHeterojunction
VUV-PCO
Catalytic ozonation
Ozone decomposition
Photocatalytic mechanism
Issue Date2019
PublisherElsevier BV. The Journal's web site is located at http://www.elsevier.com/locate/apcatb
Citation
Applied Catalysis B: Environmental, 2019, v. 259, p. article no. 118034 How to Cite?
AbstractA series of TiO2/MnO2 heterojunction catalysts were fabricated through an in-situ hydrothermal method, and for the first time, catalysts with this heterojunction structure were used for VUV-PCO toluene degradation. After the MnO2 coating, the TiO2/MnO2 catalysts performed excellently for both VOCs degradation and residual ozone decomposition with removal efficiency reaching 96.0% and 99.9%, respectively. The enhanced photocatalytic activity towards toluene degradation could be attributed to the heterojunction structure of TiO2/MnO2, which provides excellent contact between MnO2 and TiO2, and suppresses the recombination of photogenerated electron-hole pairs. Moreover, benefiting from the MnO2, the ozone generated in the system could be efficiently utilized and eliminated during the VUV-PCO process. The photocatalytic mechanism of TiO2/MnO2 for the toluene degradation and ozone decomposition was proposed.
Persistent Identifierhttp://hdl.handle.net/10722/300600
ISSN
2023 Impact Factor: 20.2
2023 SCImago Journal Rankings: 5.112
ISI Accession Number ID

 

DC FieldValueLanguage
dc.contributor.authorZHANG, Y-
dc.contributor.authorWU, M-
dc.contributor.authorKWOK, YH-
dc.contributor.authorWANG, Y-
dc.contributor.authorZhao, W-
dc.contributor.authorZHAO, X-
dc.contributor.authorHuang, H-
dc.contributor.authorLeung, DYC-
dc.date.accessioned2021-06-18T14:54:19Z-
dc.date.available2021-06-18T14:54:19Z-
dc.date.issued2019-
dc.identifier.citationApplied Catalysis B: Environmental, 2019, v. 259, p. article no. 118034-
dc.identifier.issn0926-3373-
dc.identifier.urihttp://hdl.handle.net/10722/300600-
dc.description.abstractA series of TiO2/MnO2 heterojunction catalysts were fabricated through an in-situ hydrothermal method, and for the first time, catalysts with this heterojunction structure were used for VUV-PCO toluene degradation. After the MnO2 coating, the TiO2/MnO2 catalysts performed excellently for both VOCs degradation and residual ozone decomposition with removal efficiency reaching 96.0% and 99.9%, respectively. The enhanced photocatalytic activity towards toluene degradation could be attributed to the heterojunction structure of TiO2/MnO2, which provides excellent contact between MnO2 and TiO2, and suppresses the recombination of photogenerated electron-hole pairs. Moreover, benefiting from the MnO2, the ozone generated in the system could be efficiently utilized and eliminated during the VUV-PCO process. The photocatalytic mechanism of TiO2/MnO2 for the toluene degradation and ozone decomposition was proposed.-
dc.languageeng-
dc.publisherElsevier BV. The Journal's web site is located at http://www.elsevier.com/locate/apcatb-
dc.relation.ispartofApplied Catalysis B: Environmental-
dc.subjectHeterojunction-
dc.subjectVUV-PCO-
dc.subjectCatalytic ozonation-
dc.subjectOzone decomposition-
dc.subjectPhotocatalytic mechanism-
dc.titleIn-situ synthesis of heterojunction TiO2/MnO2 nanostructure with excellent performance in vacuum ultraviolet photocatalytic oxidation of toluene-
dc.typeArticle-
dc.identifier.emailLeung, DYC: ycleung@hku.hk-
dc.identifier.authorityLeung, DYC=rp00149-
dc.description.naturelink_to_subscribed_fulltext-
dc.identifier.doi10.1016/j.apcatb.2019.118034-
dc.identifier.scopuseid_2-s2.0-85070594147-
dc.identifier.hkuros323028-
dc.identifier.volume259-
dc.identifier.spagearticle no. 118034-
dc.identifier.epagearticle no. 118034-
dc.identifier.isiWOS:000488308800011-
dc.publisher.placeNetherlands-

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