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Article: Thermal Regulation of Colloidal Materials Architecture through Orthogonal Functionalizable Patchy Particles

TitleThermal Regulation of Colloidal Materials Architecture through Orthogonal Functionalizable Patchy Particles
Authors
Wang, YuZheng, XiaolongWang, YufengPine, David J.Weck, Marcus
Issue Date2016
Citation
Chemistry of Materials, 2016, v. 28, n. 11, p. 3984-3989 How to Cite?
DOI: http://dx.doi.org/10.1021/acs.chemmater.6b01313
Abstract© 2016 American Chemical Society.This contribution presents a sol-gel based cluster encapsulation methodology to produce bifunctional patchy particles. The particles possess azide moieties on the surfaces of the patch and carboxylic acids on the shell. Two types of DNA with distinct terminal sequences are site-specifically conjugated to the particle patches or the shell employing two orthogonal coupling strategies: strain-promoted alkyne-azide cycloaddition and carbodiimide-mediated amidation. We can activate and deactivate assembly on the patches and/or the shell through thermal control, demonstrating reversible and stepwise self-assembly.
Persistent Identifierhttp://hdl.handle.net/10722/230634
ISSN
0897-4756
2023 Impact Factor: 7.2
2023 SCImago Journal Rankings: 2.421
ISI Accession Number ID
WOS:000378016400052

 

DC FieldValueLanguage
dc.contributor.authorWang, Yu-
dc.contributor.authorZheng, Xiaolong-
dc.contributor.authorWang, Yufeng-
dc.contributor.authorPine, David J.-
dc.contributor.authorWeck, Marcus-
dc.date.accessioned2016-09-01T06:06:25Z-
dc.date.available2016-09-01T06:06:25Z-
dc.date.issued2016-
dc.identifier.citationChemistry of Materials, 2016, v. 28, n. 11, p. 3984-3989-
dc.identifier.issn0897-4756-
dc.identifier.urihttp://hdl.handle.net/10722/230634-
dc.description.abstract© 2016 American Chemical Society.This contribution presents a sol-gel based cluster encapsulation methodology to produce bifunctional patchy particles. The particles possess azide moieties on the surfaces of the patch and carboxylic acids on the shell. Two types of DNA with distinct terminal sequences are site-specifically conjugated to the particle patches or the shell employing two orthogonal coupling strategies: strain-promoted alkyne-azide cycloaddition and carbodiimide-mediated amidation. We can activate and deactivate assembly on the patches and/or the shell through thermal control, demonstrating reversible and stepwise self-assembly.-
dc.languageeng-
dc.relation.ispartofChemistry of Materials-
dc.titleThermal Regulation of Colloidal Materials Architecture through Orthogonal Functionalizable Patchy Particles-
dc.typeArticle-
dc.description.naturelink_to_subscribed_fulltext-
dc.identifier.doi10.1021/acs.chemmater.6b01313-
dc.identifier.scopuseid_2-s2.0-84975076504-
dc.identifier.volume28-
dc.identifier.issue11-
dc.identifier.spage3984-
dc.identifier.epage3989-
dc.identifier.eissn1520-5002-
dc.identifier.isiWOS:000378016400052-
dc.identifier.issnl0897-4756-

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