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- Publisher Website: 10.1016/0013-4686(88)85012-6
- Scopus: eid_2-s2.0-1242307657
- WOS: WOS:A1988R441400010
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Article: Meniscus behavior and oxygen reduction in tapered pore gas diffusion electrodes
Title | Meniscus behavior and oxygen reduction in tapered pore gas diffusion electrodes |
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Authors | |
Issue Date | 1988 |
Publisher | Pergamon. The Journal's web site is located at http://www.elsevier.com/locate/electacta |
Citation | Electrochimica Acta, 1988, v. 33 n. 12, p. 1767-1773 How to Cite? |
Abstract | The electrochemical reduction of oxygen in 0.88 M KOH at 25°C was studied using two silver plated copper electrodes that contained uniform, parallel, tapered pores. Photolithography, etching, and plating techniques were used to fabricate these electrodes. Exchange current densities of 2 × 10-5 A cm-2 and 2 × 10-6 A cm-2 were measured using an initial slope method. Diffusion limiting currents increased with differential pressure across the gas-electrolyte interface which suggests smaller contact angles at higher pressures. A wedge meniscus model that treats activation, ohmic, and concentration overpotential was applied to fit the polarization curves. © 1988. |
Persistent Identifier | http://hdl.handle.net/10722/167885 |
ISSN | 2023 Impact Factor: 5.5 2023 SCImago Journal Rankings: 1.159 |
ISI Accession Number ID |
DC Field | Value | Language |
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dc.contributor.author | Chan, KY | en_US |
dc.contributor.author | Cocchetto, JF | en_US |
dc.contributor.author | Efthymiou, GS | en_US |
dc.date.accessioned | 2012-10-08T03:12:31Z | - |
dc.date.available | 2012-10-08T03:12:31Z | - |
dc.date.issued | 1988 | en_US |
dc.identifier.citation | Electrochimica Acta, 1988, v. 33 n. 12, p. 1767-1773 | en_US |
dc.identifier.issn | 0013-4686 | en_US |
dc.identifier.uri | http://hdl.handle.net/10722/167885 | - |
dc.description.abstract | The electrochemical reduction of oxygen in 0.88 M KOH at 25°C was studied using two silver plated copper electrodes that contained uniform, parallel, tapered pores. Photolithography, etching, and plating techniques were used to fabricate these electrodes. Exchange current densities of 2 × 10-5 A cm-2 and 2 × 10-6 A cm-2 were measured using an initial slope method. Diffusion limiting currents increased with differential pressure across the gas-electrolyte interface which suggests smaller contact angles at higher pressures. A wedge meniscus model that treats activation, ohmic, and concentration overpotential was applied to fit the polarization curves. © 1988. | en_US |
dc.language | eng | en_US |
dc.publisher | Pergamon. The Journal's web site is located at http://www.elsevier.com/locate/electacta | en_US |
dc.relation.ispartof | Electrochimica Acta | en_US |
dc.title | Meniscus behavior and oxygen reduction in tapered pore gas diffusion electrodes | en_US |
dc.type | Article | en_US |
dc.identifier.email | Chan, KY:hrsccky@hku.hk | en_US |
dc.identifier.authority | Chan, KY=rp00662 | en_US |
dc.description.nature | link_to_subscribed_fulltext | en_US |
dc.identifier.doi | 10.1016/0013-4686(88)85012-6 | - |
dc.identifier.scopus | eid_2-s2.0-1242307657 | en_US |
dc.identifier.volume | 33 | en_US |
dc.identifier.issue | 12 | en_US |
dc.identifier.spage | 1767 | en_US |
dc.identifier.epage | 1773 | en_US |
dc.identifier.isi | WOS:A1988R441400010 | - |
dc.publisher.place | United Kingdom | en_US |
dc.identifier.scopusauthorid | Chan, KY=7406034142 | en_US |
dc.identifier.scopusauthorid | Cocchetto, JF=6506669149 | en_US |
dc.identifier.scopusauthorid | Efthymiou, GS=6602937018 | en_US |
dc.identifier.issnl | 0013-4686 | - |