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Article: Highly enantioselective synthesis of chiral secondary amines by gold(I)/ chiral bronsted acid catalyzed tandem intermodular hydroamination and transfer hydrogenation reactions

TitleHighly enantioselective synthesis of chiral secondary amines by gold(I)/ chiral bronsted acid catalyzed tandem intermodular hydroamination and transfer hydrogenation reactions
Authors
Issue Date2009
PublisherAmerican Chemical Society. The Journal's web site is located at http://pubs.acs.org/journals/orlef7/index.html
Citation
Organic Letters, 2009, v. 11 n. 18, p. 4204-4207 How to Cite?
AbstractA method for the synthesis of enantiomerically enriched secondary amines with excellent ee values through the tandem intermolecular hydroamination/ transfer hydrogenation of alkynes using a "gold(I) complex-chiral Brønsted acid" protocol is developed. The catalysis works for a wide variety of aryl, alkenyl, and aliphatic alkynes as well as anilines with different electronic properties. © 2009 American Chemical Society.
Persistent Identifierhttp://hdl.handle.net/10722/70254
ISSN
2015 Impact Factor: 6.732
2015 SCImago Journal Rankings: 3.187
ISI Accession Number ID
Funding AgencyGrant Number
University of Hong Kong
Hong Kong Research Grants CouncilHKU 1/CRF/08
HKU 7007/08P
University Grants Committee of Hong KongAoE/P-10/01
Funding Information:

We are thankful for the financial support of The University of Hong Kong (University Development Fund), Hong Kong Research Grants Council (HKU 1/CRF/08, HKU 7007/08P), and University Grants Committee of Hong Kong (Areas of Excellence Scheme AoE/P-10/01).

References
Grants

 

DC FieldValueLanguage
dc.contributor.authorLiu, XYen_HK
dc.contributor.authorChe, CMen_HK
dc.date.accessioned2010-09-06T06:21:09Z-
dc.date.available2010-09-06T06:21:09Z-
dc.date.issued2009en_HK
dc.identifier.citationOrganic Letters, 2009, v. 11 n. 18, p. 4204-4207en_HK
dc.identifier.issn1523-7060en_HK
dc.identifier.urihttp://hdl.handle.net/10722/70254-
dc.description.abstractA method for the synthesis of enantiomerically enriched secondary amines with excellent ee values through the tandem intermolecular hydroamination/ transfer hydrogenation of alkynes using a "gold(I) complex-chiral Brønsted acid" protocol is developed. The catalysis works for a wide variety of aryl, alkenyl, and aliphatic alkynes as well as anilines with different electronic properties. © 2009 American Chemical Society.en_HK
dc.languageengen_HK
dc.publisherAmerican Chemical Society. The Journal's web site is located at http://pubs.acs.org/journals/orlef7/index.htmlen_HK
dc.relation.ispartofOrganic Lettersen_HK
dc.subject.meshAlkynes - chemistry-
dc.subject.meshAmines - chemical synthesis-
dc.subject.meshAniline Compounds - chemistry-
dc.subject.meshGold - chemistry-
dc.subject.meshStereoisomerism-
dc.titleHighly enantioselective synthesis of chiral secondary amines by gold(I)/ chiral bronsted acid catalyzed tandem intermodular hydroamination and transfer hydrogenation reactionsen_HK
dc.typeArticleen_HK
dc.identifier.openurlhttp://library.hku.hk:4550/resserv?sid=HKU:IR&issn=1523-7060&volume=11&issue=18&spage=4204&epage=4207&date=2009&atitle=Highly+enantioselective+synthesis+of+chiral+secondary+amines+by+gold+(I)/+chiral+Brønsted+acid+catalyzed+tandem+intermolecular+hydroamination+and+transfer+hydrogenation+reactionsen_HK
dc.identifier.emailChe, CM:cmche@hku.hken_HK
dc.identifier.authorityChe, CM=rp00670en_HK
dc.description.naturelink_to_subscribed_fulltext-
dc.identifier.doi10.1021/ol901443ben_HK
dc.identifier.pmid19678678-
dc.identifier.scopuseid_2-s2.0-70349147881en_HK
dc.identifier.hkuros168981en_HK
dc.relation.referenceshttp://www.scopus.com/mlt/select.url?eid=2-s2.0-70349147881&selection=ref&src=s&origin=recordpageen_HK
dc.identifier.volume11en_HK
dc.identifier.issue18en_HK
dc.identifier.spage4204en_HK
dc.identifier.epage4207en_HK
dc.identifier.isiWOS:000269670700045-
dc.publisher.placeUnited Statesen_HK
dc.relation.projectInstitute of molecular technology for drug discovery and synthesis-
dc.identifier.scopusauthoridLiu, XY=27171788000en_HK
dc.identifier.scopusauthoridChe, CM=7102442791en_HK
dc.identifier.citeulike9067278-

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