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Article: Amidation of saturated C-H bonds catalyzed by electron-deficient ruthenium and manganese porphyrins. A highly catalytic nitrogen atom transfer process

TitleAmidation of saturated C-H bonds catalyzed by electron-deficient ruthenium and manganese porphyrins. A highly catalytic nitrogen atom transfer process
Authors
Issue Date2000
PublisherAmerican Chemical Society. The Journal's web site is located at http://pubs.acs.org/journals/orlef7/index.html
Citation
Organic Letters, 2000, v. 2 n. 15, p. 2233-2236 How to Cite?
Abstract(equation presented) Amidation of a variety of hydrocarbons with PhI=NTs catalyzed by ruthenium and manganese meso-tetrakis(pentafluorophenyl)porphyrins 1 and 2 afforded N-substituted amides in up to 92% yields with good to excellent substrate conversions. By employing catalyst 2, exceptionally high turnovers (up to 2600) were achieved, and the amidations can be effected by directly using PhI(OAc)2/NH2R as amidating reagents; in the case of R = COCF3 a direct amination was realized in up to 90% yield.
Persistent Identifierhttp://hdl.handle.net/10722/69077
ISSN
2015 Impact Factor: 6.732
2015 SCImago Journal Rankings: 3.187
ISI Accession Number ID
References

 

DC FieldValueLanguage
dc.contributor.authorYu, XQen_HK
dc.contributor.authorHuang, JSen_HK
dc.contributor.authorZhou, XGen_HK
dc.contributor.authorChe, CMen_HK
dc.date.accessioned2010-09-06T06:10:21Z-
dc.date.available2010-09-06T06:10:21Z-
dc.date.issued2000en_HK
dc.identifier.citationOrganic Letters, 2000, v. 2 n. 15, p. 2233-2236en_HK
dc.identifier.issn1523-7060en_HK
dc.identifier.urihttp://hdl.handle.net/10722/69077-
dc.description.abstract(equation presented) Amidation of a variety of hydrocarbons with PhI=NTs catalyzed by ruthenium and manganese meso-tetrakis(pentafluorophenyl)porphyrins 1 and 2 afforded N-substituted amides in up to 92% yields with good to excellent substrate conversions. By employing catalyst 2, exceptionally high turnovers (up to 2600) were achieved, and the amidations can be effected by directly using PhI(OAc)2/NH2R as amidating reagents; in the case of R = COCF3 a direct amination was realized in up to 90% yield.en_HK
dc.languageengen_HK
dc.publisherAmerican Chemical Society. The Journal's web site is located at http://pubs.acs.org/journals/orlef7/index.htmlen_HK
dc.relation.ispartofOrganic Lettersen_HK
dc.titleAmidation of saturated C-H bonds catalyzed by electron-deficient ruthenium and manganese porphyrins. A highly catalytic nitrogen atom transfer processen_HK
dc.typeArticleen_HK
dc.identifier.openurlhttp://library.hku.hk:4550/resserv?sid=HKU:IR&issn=1523-7060&volume=2&issue=15&spage=2233&epage=2236&date=2000&atitle=Amidation+of+saturated+C-H+bonds+catalyzed+by+electron-deficient+ruthenium+and+manganese+porphyrins.++A+highly+catalytic+nitrogen+atom+transfer+processen_HK
dc.identifier.emailHuang, JS:jshuang@hkucc.hku.hken_HK
dc.identifier.emailChe, CM:cmche@hku.hken_HK
dc.identifier.authorityHuang, JS=rp00709en_HK
dc.identifier.authorityChe, CM=rp00670en_HK
dc.description.naturelink_to_subscribed_fulltext-
dc.identifier.doi10.1021/ol000107r-
dc.identifier.pmid10930251en_HK
dc.identifier.scopuseid_2-s2.0-0034720956en_HK
dc.identifier.hkuros64755en_HK
dc.relation.referenceshttp://www.scopus.com/mlt/select.url?eid=2-s2.0-0034720956&selection=ref&src=s&origin=recordpageen_HK
dc.identifier.volume2en_HK
dc.identifier.issue15en_HK
dc.identifier.spage2233en_HK
dc.identifier.epage2236en_HK
dc.identifier.isiWOS:000088346400014-
dc.publisher.placeUnited Statesen_HK
dc.identifier.scopusauthoridYu, XQ=37861478700en_HK
dc.identifier.scopusauthoridHuang, JS=7407192639en_HK
dc.identifier.scopusauthoridZhou, XG=37105544400en_HK
dc.identifier.scopusauthoridChe, CM=7102442791en_HK

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