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Article: Gold(III) (C^N) complex-catalyzed synthesis of propargylamines via a three-component coupling reaction of aldehydes, amines and alkynes
Title | Gold(III) (C^N) complex-catalyzed synthesis of propargylamines via a three-component coupling reaction of aldehydes, amines and alkynes | ||||||||||
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Authors | |||||||||||
Keywords | Gold(III) catalyst Prolinol derivatives Propargylamines Three-component coupling reaction | ||||||||||
Issue Date | 2009 | ||||||||||
Publisher | Elsevier SA. The Journal's web site is located at http://www.elsevier.com/locate/jorganchem | ||||||||||
Citation | Journal Of Organometallic Chemistry, 2009, v. 694 n. 4, p. 583-591 How to Cite? | ||||||||||
Abstract | Propargylamines are synthesized in high yields via a gold(III) (C^N) complex-catalyzed three-component coupling reaction of aldehydes, amines and alkynes in water at 40 °C. Excellent diastereoselectivities (up to 99:1) have been achieved when chiral prolinol derivatives are employed as the amine component. Notably, the [Au(C^N)Cl2] complex (N^CH = 2-phenylpyridine) could be repeatedly used for 10 reaction cycles, leading to an overall turnover number of 812. © 2008 Elsevier B.V. All rights reserved. | ||||||||||
Persistent Identifier | http://hdl.handle.net/10722/58333 | ||||||||||
ISSN | 2023 Impact Factor: 2.1 2023 SCImago Journal Rankings: 0.359 | ||||||||||
ISI Accession Number ID |
Funding Information: This work was supported by the Hong Kong Research Grants Council (PolyU 7052/07P), PolyU Departmental General Research Funds, The University of Hong Kong (University Development Fund), and the University Grants Committee of the Hong Kong SAR of China (Area of Excellence Scheme, AoE/P-10/01). | ||||||||||
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Grants |
DC Field | Value | Language |
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dc.contributor.author | Lo, VKY | en_HK |
dc.contributor.author | Kung, KKY | en_HK |
dc.contributor.author | Wong, MK | en_HK |
dc.contributor.author | Che, CM | en_HK |
dc.date.accessioned | 2010-05-31T03:28:28Z | - |
dc.date.available | 2010-05-31T03:28:28Z | - |
dc.date.issued | 2009 | en_HK |
dc.identifier.citation | Journal Of Organometallic Chemistry, 2009, v. 694 n. 4, p. 583-591 | en_HK |
dc.identifier.issn | 0022-328X | en_HK |
dc.identifier.uri | http://hdl.handle.net/10722/58333 | - |
dc.description.abstract | Propargylamines are synthesized in high yields via a gold(III) (C^N) complex-catalyzed three-component coupling reaction of aldehydes, amines and alkynes in water at 40 °C. Excellent diastereoselectivities (up to 99:1) have been achieved when chiral prolinol derivatives are employed as the amine component. Notably, the [Au(C^N)Cl2] complex (N^CH = 2-phenylpyridine) could be repeatedly used for 10 reaction cycles, leading to an overall turnover number of 812. © 2008 Elsevier B.V. All rights reserved. | en_HK |
dc.language | eng | en_HK |
dc.publisher | Elsevier SA. The Journal's web site is located at http://www.elsevier.com/locate/jorganchem | en_HK |
dc.relation.ispartof | Journal of Organometallic Chemistry | en_HK |
dc.subject | Gold(III) catalyst | en_HK |
dc.subject | Prolinol derivatives | en_HK |
dc.subject | Propargylamines | en_HK |
dc.subject | Three-component coupling reaction | en_HK |
dc.title | Gold(III) (C^N) complex-catalyzed synthesis of propargylamines via a three-component coupling reaction of aldehydes, amines and alkynes | en_HK |
dc.type | Article | en_HK |
dc.identifier.openurl | http://library.hku.hk:4550/resserv?sid=HKU:IR&issn=0022-328X&volume=694&spage=583&epage=591&date=2009&atitle=Gold(III)+(C^N)+Complex-Catalyzed+Synthesis+of+Propargylamines+via+a+Three-Component+Coupling+Reaction+of+Aldehydes,+Amines+and+Alkynes+ | en_HK |
dc.identifier.email | Che, CM:cmche@hku.hk | en_HK |
dc.identifier.authority | Che, CM=rp00670 | en_HK |
dc.description.nature | link_to_subscribed_fulltext | - |
dc.identifier.doi | 10.1016/j.jorganchem.2008.12.008 | en_HK |
dc.identifier.scopus | eid_2-s2.0-58649115594 | en_HK |
dc.identifier.hkuros | 155987 | en_HK |
dc.identifier.hkuros | 177355 | - |
dc.relation.references | http://www.scopus.com/mlt/select.url?eid=2-s2.0-58649115594&selection=ref&src=s&origin=recordpage | en_HK |
dc.identifier.volume | 694 | en_HK |
dc.identifier.issue | 4 | en_HK |
dc.identifier.spage | 583 | en_HK |
dc.identifier.epage | 591 | en_HK |
dc.identifier.isi | WOS:000262887200017 | - |
dc.publisher.place | Switzerland | en_HK |
dc.relation.project | Institute of molecular technology for drug discovery and synthesis | - |
dc.identifier.scopusauthorid | Lo, VKY=13406071200 | en_HK |
dc.identifier.scopusauthorid | Kung, KKY=25959176500 | en_HK |
dc.identifier.scopusauthorid | Wong, MK=7403908449 | en_HK |
dc.identifier.scopusauthorid | Che, CM=7102442791 | en_HK |
dc.identifier.issnl | 0022-328X | - |