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Article: Effects of volume evolution of static and dynamic polar nanoregions on the dielectric behavior of relaxors

TitleEffects of volume evolution of static and dynamic polar nanoregions on the dielectric behavior of relaxors
Authors
KeywordsBulk permittivity
Correlation strength
Curie weiss law
Dielectric behavior
Dielectric response
Issue Date2011
PublisherAmerican Institute of Physics. The Journal's web site is located at http://apl.aip.org/
Citation
Applied Physics Letters, 2011, v. 99 n. 9, article no. 092908 How to Cite?
AbstractRecent experiments revealed unusual dielectric behaviors of Pb(Mg 1/3Nb 2/3)O 3 originated from polar nanoregions (PNRs). Thus, Pauli's master equation is adopted to investigate the distinct dielectric responses, correlation strength, and volume evolutions of static and dynamic PNRs. Our findings have not only validated the percolation theory but also ascertained Lorentzian distribution of the rate of thermal change of PNR volume. Finally, based on Maxwell's equation the observed dielectric deviations of bulk permittivity from Curie-Weiss law are attributed to the thermal effects on static volume fraction and polarization rotation. © 2011 American Institute of Physics.
Persistent Identifierhttp://hdl.handle.net/10722/157139
ISSN
2021 Impact Factor: 3.971
2020 SCImago Journal Rankings: 1.182
ISI Accession Number ID
Funding AgencyGrant Number
Research Grants Council of the Hong Kong Special Administrative RegionHKU 716508E
HKU 717011E
Funding Information:

Research Grants Council of the Hong Kong Special Administrative Region, under Project Nos. HKU 716508E and HKU 717011E, is acknowledged. We thank Prof. G.J. Weng at Rutgers University for helpful discussions.

References
Grants

 

DC FieldValueLanguage
dc.contributor.authorShi, YPen_US
dc.contributor.authorSoh, AKen_US
dc.date.accessioned2012-08-08T08:45:29Z-
dc.date.available2012-08-08T08:45:29Z-
dc.date.issued2011en_US
dc.identifier.citationApplied Physics Letters, 2011, v. 99 n. 9, article no. 092908-
dc.identifier.issn0003-6951en_US
dc.identifier.urihttp://hdl.handle.net/10722/157139-
dc.description.abstractRecent experiments revealed unusual dielectric behaviors of Pb(Mg 1/3Nb 2/3)O 3 originated from polar nanoregions (PNRs). Thus, Pauli's master equation is adopted to investigate the distinct dielectric responses, correlation strength, and volume evolutions of static and dynamic PNRs. Our findings have not only validated the percolation theory but also ascertained Lorentzian distribution of the rate of thermal change of PNR volume. Finally, based on Maxwell's equation the observed dielectric deviations of bulk permittivity from Curie-Weiss law are attributed to the thermal effects on static volume fraction and polarization rotation. © 2011 American Institute of Physics.en_US
dc.languageengen_US
dc.publisherAmerican Institute of Physics. The Journal's web site is located at http://apl.aip.org/en_US
dc.relation.ispartofApplied Physics Lettersen_US
dc.rightsCopyright 2011 American Institute of Physics. This article may be downloaded for personal use only. Any other use requires prior permission of the author and the American Institute of Physics. The following article appeared in Applied Physics Letters, 2011, v. 99 n. 9, article no. 092908 and may be found at https://doi.org/10.1063/1.3632082-
dc.subjectBulk permittivity-
dc.subjectCorrelation strength-
dc.subjectCurie weiss law-
dc.subjectDielectric behavior-
dc.subjectDielectric response-
dc.titleEffects of volume evolution of static and dynamic polar nanoregions on the dielectric behavior of relaxorsen_US
dc.typeArticleen_US
dc.identifier.emailSoh, AK: aksoh@hkucc.hku.hken_US
dc.identifier.authoritySoh, AK=rp00170en_US
dc.description.naturepublished_or_final_versionen_US
dc.identifier.doi10.1063/1.3632082en_US
dc.identifier.scopuseid_2-s2.0-80052526278en_US
dc.identifier.hkuros200549-
dc.relation.referenceshttp://www.scopus.com/mlt/select.url?eid=2-s2.0-80052526278&selection=ref&src=s&origin=recordpageen_US
dc.identifier.volume99en_US
dc.identifier.issue9-
dc.identifier.spagearticle no. 092908-
dc.identifier.epagearticle no. 092908-
dc.identifier.eissn1077-3118-
dc.identifier.isiWOS:000294489300056-
dc.publisher.placeUnited Statesen_US
dc.relation.projectMulti-scale investigation of interface dominated multiferroic nanostructures (IDMNS) and exploration of potential applications-
dc.relation.projectMesoscopic study of magnetoelectroelastic coupling in multiferroic materials-
dc.identifier.scopusauthoridSoh, AK=7006795203en_US
dc.identifier.scopusauthoridShi, YP=12345267700en_US
dc.identifier.issnl0003-6951-

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