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Article: Organic diagenesis in sediment and its impact on the adsorption of bisphenol A and nonylphenol onto marine sediment

TitleOrganic diagenesis in sediment and its impact on the adsorption of bisphenol A and nonylphenol onto marine sediment
Authors
Fei, YHLi, XDLi, XY
KeywordsAdsorption
Diagenesis
EDCs
Marine water quality
Organic matter
Sediment
Issue Date2011
PublisherPergamon. The Journal's web site is located at http://www.elsevier.com/locate/marpolbul
Citation
Marine Pollution Bulletin, 2011, v. 63 n. 5-12, p. 578-582 How to Cite?
DOI: http://dx.doi.org/10.1016/j.marpolbul.2010.11.020
AbstractHydrophobic organic contaminants in marine water are mostly adsorbed onto (partitioned into) sediment organic matter (SOM). To study the impact of SOM diagenesis on sediment adsorption properties, artificial sediment with rich SOM content was incubated for more than 120. days. The sediment was sampled every week, and batch sediment adsorption tests were conducted with bisphenol A (BPA) and nonylphenol (NP) as the model pollutants. The results show that the amount of organic matter loaded in the sediment decreased by nearly 80% during incubation. For the incubated sediment, the BPA partition coefficient, Kd, decreased whereas the organic normalized partition coefficient, Koc, more than doubled. The experiments with NP show an even greater increase in Koc. Organic matter diagenesis shows a profound effect on the adsorption behavior of sediment, as the SOM residue has an increasing affinity and partition capacity for organic contaminants. © 2010 Elsevier Ltd.
Persistent Identifierhttp://hdl.handle.net/10722/137240
ISSN
0025-326X
2021 Impact Factor: 7.001
2020 SCImago Journal Rankings: 1.548
ISI Accession Number ID
WOS:000294092700075
Funding AgencyGrant Number
University Grants Council of the Government of the Hong Kong SAR, ChinaSEG-HKU10
AoE/P-04/2004
Funding Information:

This research was supported by grants SEG-HKU10 and AoE/P-04/2004 from the University Grants Council of the Government of the Hong Kong SAR, China. The technical assistance of Mr. Keith C.H. Wong is highly appreciated.

References
References in Scopus

 

DC FieldValueLanguage
dc.contributor.authorFei, YHen_HK
dc.contributor.authorLi, XDen_HK
dc.contributor.authorLi, XYen_HK
dc.date.accessioned2011-08-26T14:21:40Z-
dc.date.available2011-08-26T14:21:40Z-
dc.date.issued2011en_HK
dc.identifier.citationMarine Pollution Bulletin, 2011, v. 63 n. 5-12, p. 578-582en_HK
dc.identifier.issn0025-326Xen_HK
dc.identifier.urihttp://hdl.handle.net/10722/137240-
dc.description.abstractHydrophobic organic contaminants in marine water are mostly adsorbed onto (partitioned into) sediment organic matter (SOM). To study the impact of SOM diagenesis on sediment adsorption properties, artificial sediment with rich SOM content was incubated for more than 120. days. The sediment was sampled every week, and batch sediment adsorption tests were conducted with bisphenol A (BPA) and nonylphenol (NP) as the model pollutants. The results show that the amount of organic matter loaded in the sediment decreased by nearly 80% during incubation. For the incubated sediment, the BPA partition coefficient, Kd, decreased whereas the organic normalized partition coefficient, Koc, more than doubled. The experiments with NP show an even greater increase in Koc. Organic matter diagenesis shows a profound effect on the adsorption behavior of sediment, as the SOM residue has an increasing affinity and partition capacity for organic contaminants. © 2010 Elsevier Ltd.en_HK
dc.languageengen_US
dc.publisherPergamon. The Journal's web site is located at http://www.elsevier.com/locate/marpolbulen_HK
dc.relation.ispartofMarine Pollution Bulletinen_HK
dc.rightsNOTICE: this is the author’s version of a work that was accepted for publication in Marine Pollution Bulletin. Changes resulting from the publishing process, such as peer review, editing, corrections, structural formatting, and other quality control mechanisms may not be reflected in this document. Changes may have been made to this work since it was submitted for publication. A definitive version was subsequently published in Marine Pollution Bulletin, 2011, v. 63 n. 5-12, p. 578-582. DOI: 10.1016/j.marpolbul.2010.11.020-
dc.rightsThis work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International License.-
dc.subjectAdsorption-
dc.subjectDiagenesis-
dc.subjectEDCs-
dc.subjectMarine water quality-
dc.subjectOrganic matter-
dc.subjectSediment-
dc.subject.meshAdsorptionen_HK
dc.subject.meshEnvironmental Monitoringen_HK
dc.subject.meshGeologic Sediments - chemistryen_HK
dc.subject.meshPhenols - analysis - chemistryen_HK
dc.subject.meshSeawater - chemistryen_HK
dc.subject.meshWater Pollutants, Chemical - analysis - chemistryen_HK
dc.titleOrganic diagenesis in sediment and its impact on the adsorption of bisphenol A and nonylphenol onto marine sedimenten_HK
dc.typeArticleen_HK
dc.identifier.emailLi, XY:xlia@hkucc.hku.hken_HK
dc.identifier.authorityLi, XY=rp00222en_HK
dc.description.naturepostprint-
dc.identifier.doi10.1016/j.marpolbul.2010.11.020en_HK
dc.identifier.pmid21168171-
dc.identifier.scopuseid_2-s2.0-79960373714en_HK
dc.identifier.hkuros190471en_US
dc.relation.referenceshttp://www.scopus.com/mlt/select.url?eid=2-s2.0-79960373714&selection=ref&src=s&origin=recordpageen_HK
dc.identifier.volume63en_HK
dc.identifier.issue5-12en_HK
dc.identifier.spage578en_HK
dc.identifier.epage582en_HK
dc.identifier.isiWOS:000294092700075-
dc.publisher.placeUnited Kingdomen_HK
dc.identifier.scopusauthoridFei, YH=43061079900en_HK
dc.identifier.scopusauthoridLi, XD=43061226900en_HK
dc.identifier.scopusauthoridLi, XY=26642887900en_HK
dc.identifier.citeulike8451649-
dc.identifier.issnl0025-326X-

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